The goal of Dr. Kleiman's thesis was to measure and,
thereby, deduce the emissions of some trace short-lived reactive
organochlorine gases which have health and environmental
implications. For this effort, he personally designed and installed
a complex automated instrument at a field station in Nahant to yield
a unique dataset of high-frequency concentration measurements for
these gases. He then utilized an innovative approach using
calculated Lagrangian back-trajectories and a recursive weighted
least squares filter to deduce regional emissions of these gases. He
then compared these emissions to those deduced from industry
information. He demonstrated that this new approach provides an
important independent observation-based method for deducing regional
emissions. He showed that this method yielded reasonable agreement
with industry-based estimates in some but not all cases, thus
pinpointing possible errors in the industry-based approach. With
this work, Gary Kleiman has shown the capability to work all the way
from producing difficult yet very high quality observations, to a
theoretical analysis of these measurements to yield a new approach
for deducing regional emissions of short-lived environmentally
important trace gases. This combination of accomplishments deserves
the special recognition of the Rossby Award.